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Essential oils from four Cistus species (C. setosus L., C. ladanifer L., C. salviifolius Turra and C. monspeliensis L.) were isolated and analyzed by GC-FID and GC-MS. Quantitative analysis of the main compounds was performed by GC-FID. Principal component analysis was performed to assess the similarities among these essential oils, and the antioxidant activity of the oils was tested on radical scavenging activities of DPPH and ABTS radicals. The oils contain mainly monoterpene hydrocarbons and oxygenated monoterpenes in different proportions, depending on the species, with the predominance of (+)-(S)-linalool in C. setosus L., 1,8-cineole in C. salviifolius, alpha-terpineol and alpha-terpinyl acetate in C. monspeliensis and linalool in C. ladanifer. This work reports, for the first time, the antioxidant activity of the Cistus essential oils. All these oils exhibit important antioxidant activity, with IC(50) values ranging from 6.2 to 12.1 microL/mL, corresponding to the concentration of 50 microg/mL. The activity of the oils on the DPPH radical was in the order of effectiveness: C. setosus L. > C. salviifolius > C. monspeliensis > C. ladanifer. Moreover, the C. setosus L. oil scavenged more effectively than the C. ladanifer oil, which is of great interest considering the very low content of linalool (0.1%) in this species. The antioxidant activity of
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