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The binding of transition metal ions (ScIII, CrIV, MnIV, CoII, CuII, NiII, PdII and ZnII) to 4,6-diazacyclo[5.5.0.0]undec-9-ene (NDACU) was investigated by spectrophotometric method in chloroform medium. The stability constants of the complexes were calculated from the spectral changes observed in different concentration of ligand and the binding of the metal ions to NDACU were followed with the help of MIR, UV-Vis and (1)H NMR techniques. The binding constants were also calculated by using Benesi-Hildebrand equation and the stability constants were found to be in the range of 105.5-475.5. The lowest stability constants of NDACU-TM complexes were observed for PdII, CrIV and ZnII. The formation of tetra-coordinated complexes were confirmed with the help of NMR titration studies. Also the condensation of NDACU with methyl 2-phenylacetate and methyl p-tolylacetate were investigated. The stoichiometry of reaction was
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